Sonderforschungsbereich 546
"Struktur, Dynamik und Reaktivität von
Übergangsmetalloxid-Aggregaten"
Publikationen im TP A3:
Berichtszeitraum 2008/2 - 2011/1
- [LMD11]
- S. Li, A. Mirabal, J. Demuth, L. Wöste and T. Siebert
On the Role of Thermal Activation in Selective Photochemistry: Mechanistic Insight to the Oxidation of Propene on the V4O11-
Phys. Chem. Chem. Phys.
14 (2012) 148 - 156.
- [BWS11]
- A.M. Burow, T. Wende, M. Sierka, R. Wlodarczyk, J. Sauer,
P. Claes, L. Jiang, G. Meijer, P. Lievens, K.R. Asmis
Structures and Vibrational Spectroscopy of Partially Reduced Gas-Phase Cerium
Oxide Clusters
Phys. Chem. Chem. Phys.
13 (2011) 19393 - 19400.
- [JWC11]
- L. Jiang, T. Wende, P. Claes, S. Bhattacharyya, M. Sierka,
G. Meijer, P. Lievens, J. Sauer and K. R. Asmis
Electron distribution in Partially Reduced Mixed metal Oxide Systems: Infrared
Spectroscopy of CemVnOo+ Gas Phase Clusters
J. Phys. Chem. A. 115
(2011) 11187 - 11192.
- [LCH10]
- L. Lin, P. Claes, T. Höltzl,
E. Janssens, T. Wende, R. Bergmann, G. Santambrogio, G. Meijer, K.R. Asmis,
M.T. Nguyen, P. Lievens
The structure of Au6Y+in the Gas Phase
Phys. Chem. Chem. Phys.
12 (2010) 13907 - 13913.
- [WDJ10]
- T. Wende, J. Döbler, L. Jiang, P. Claes, E. Janssens,
P. Lievens, G. Meijer, K. R. Asmis and J. Sauer
Infrared spectroscopic characterization of the oxidative dehydrogenation of
propane by V4O10+
Int. J. Mass Spectrom.
297 (2010) 102 - 106.
- [SJL08]
- D. Santambrogio, E. Janssens, S. Li, T. Siebert, G. Meijer, K.R. Asmis, J. Döbler, M. Sierka and J. Sauer
Identification of Conical Structures in Small Aluminium Oxide Clusters: Infrared Spectroscopy of (Al2O3)1-4 (AlO)+
J. Am. Chem. Soc. 130 (2008) 15143 - 15149.
- [SBW08]
- G. Santambrogio, M. Brümmer, L. Wöste, J. Döbler, J. Sauer, G. Meijer and K. R. Asmis
Gas Phase Vibrational Spectroscopy of Mass-Selected Vanadium Oxide Cluster Anions
Phys. Chem. Chem. Phys. 10 (2008) 3992 - 4005.
- [LMD08]
- S. Li, A. Mirabal, J. Demuth, L. Wöste and T. Siebert
A Complete Reactant - Product Ananlysis of the Oxygen Transfer Reaction in
[V4O11·C3H6] -:
A Cluster Complex for Modeling Surface Activation and Reactivity
J. Am. Chem. Soc.
130 (2008) 16832 - 16833.
- [SUM08]
- B.E. Schmidt, W. Unrau, A. Mirabal, S. li, M. Krenz, L.
Wöste and T. Siebert
Poor man's source for sub 7 fs: a simple route to ultrashort laser pulses
and their full characterization
Opt. Express 16
(2008) 18910 - 21.
- [SJL08]
- D. Santambrogio, E. Janssens, S. Li, T. Siebert, G. Meijer, K.R. Asmis, J. Döbler, M. Sierka and J. Sauer
Identification of Conical Structures in Small Aluminium Oxide Clusters: Infrared Spectroscopy of (Al2O3)1-4 (AlO)+
J. Am. Chem. Soc. 130 (2008) 15143 - 15149.
Berichtszeitraum 2005/2 - 2008/1
- [WKL05]
- J. Weissenrieder, S. Kaya, J.-L. Lu, H.-J. Gao, S. Shaikhutdinov,
H.-J. Freund, M. Sierka, T. K. Todorova and J. Sauer Atomic Structure of a
Thin Silica Film on a Mo(112) Substrate: A Two-Dimensional Network of SiO4
Tetrahedra
Phys. Rev. Lett.
95 (2005) 076103-1 - 076103-4
Berichtszeitraum 2002/2 - 2005/1
- [KSB05]
- K. Asmis, G. Santambrogio, M. Brümmer, J. Sauer
Polyhedral Vanadium Oxide Cages: Infrared Spectra of Cluster Anions and
Size-Induced d Electron Localization
Angew. Chem. 117
(2005) 3182 ; Angew.
Chem. Int. Ed. 44 (2005) 3122
- [SBW05]
-
- G. Santambrogio, M. Brümmer, L. Wöste, J. Sauer,
G. Meijer, K. R. Asmis
Gas Phase Infrared Spectroscopy of Vanadium Oxide
Cluster Anions
- [AMB04]
- K.R. Asmis, G. Meijer, M. Brümmer, C. Kaposta, G.
Santambrogio, L. Wöste, J. Sauer
Gas Phase Infrared Spectroscopy of Mono- and Divanadium Oxide Cluster Cations
J. Chem. Phys. 120
(2004) 6461
- [NKO04]
- M.J. Nee, C. Kaposta, A. Osterwalder, C. Cibrián
Uhalte, T. Xie, A. Kaledin, S. Carter, J.M. Bowman, D.M. Neumark and K.R.
Asmis
Experimental and theoretical study of the infrared spectra of BrHI-
and BrDI-
J. Chem. Phys. 121
(2004) 7259
- [KA04]
- O. Kühn, K. Asmis
Bausteine des Wassers unter der Laserlupe fundiert
Das Wissenschaftsmagazin
der Freien Universität Berlin 2 (2004) 84
- [K04]
- K. Asmis, Gas Phase Infrared Spectroscopy of Vanadium
Oxide Cluster Ions
Symposium of the DFG Colloborative Research Center 546, 21-24 März
2004, Berlin-Schmökwitz (D)
- [APS03]
- K.R. Asmis, N.L. Pivonka, G. Santambrogio, M. Brümmer,
C. Kaposta, D.M. Neumark and L. Wöste
The Gasphase Infrared Spectrum of the Protonated Water Dimer
Science
299 (2003) 1375
- [BKS03]
- M. Brümmer, C. Kaposta, G. Santambrogio, K.R. Asmis
Formation and Photodepletion of Cluster Ion - Messenger Atom Complexes in
a Cold Ion Trap: Infrared Spectroscopy of VO+, VO2+
and VO3+
J. Chem. Phys. 119
(2003) 12700
- [PKB03]
- N.L. Pivonka, C. Kaposta, M. Brümmer, G. von Helden,
G. Meijer, L. Wöste, D.M. Neumark and K.R. Asmis
Probing a Strong Hydrogen Bond with Infrared Spectroscopy: Vibrational Predissociation
of BrHBr-.Ar
J. Chem. Phys. 118
(2003) 5275
- [ABK02]
- K.R. Asmis, M. Brümmer, C. Kaposta, G. Santambrogio,
G. von Helden, G. Meijer, K. Rademann and L. Wöste
Mass-selected Infrared Photodissociation Spectroscopy of V4O10+
Phys. Chem. Chem. Phys.
4 (2002) 1101
- [K02]
- K. Asmis, Infrared Spectroscopy of Mass-selected Gas Phase
Cluster Ions
XIth International Symposium on Small Particles and Inorganic Clusters (ISSPIC
11), 9-13 September 2002, Strasbourg (F)
- [PKH02]
- N.L. Pivonka, C. Kaposta, G. von Helden, G. Meijer, L.
Wöste, D.M. Neumark and K.R. Asmis
Gas Phase Infrared Spectroscopy of Cluster Anions as a Function of Size:
The Effect of Solvation on Hydrogen-Bonding in Br-(HBr)1,2,3
Clusters
J. Chem. Phys. 117
(2002) 6493
-
-
Berichtszeitraum 2002/2 - 2005/1
- H. Hess, K.R. Asmis, T. Leisner, L. Wöste
Vibrational Wave Packet Dynamics in the Silver Tetramer Probed by NeNePo Femtosecond
Pump-probe Spectroscopy
Euro. J. Phys. D 16 (2001) 145-149
- A. Fielicke, K. Rademann
Alkene Oxidation on Metal Oxide Clusters: Model Systems for Active Centers
In: Extended Abstracts of the 4th World
Congress on Oxidation Catalysis, Vol II, Sept. 16-21,
2001, Potsdam, Germany (2001) pp. 133-136
- J. Opitz-Coutureau, A. Fielicke, B. Kaiser, K.
Rademann
"Antimony and
Bismuth Oxide Cluster Ions"
PCCP 3 (2001) 3034-3041
- K. Rademann, A. Fielicke, A. Pramann
"Struktur und Reaktivität von Metall- und Metalloxidclustern
in der Chemie an der Humboldt-Universität zu Berlin"
100 Jahre Chemische Institute in der Hessischen
Straße, Verlag für Marketing und Kommunikation,
Worms (2000) 96-101
- A. Fielicke, K. Rademann
"Interaction of
Bismuth Oxide Cluster Cations with Alkenes and Molecular Oxygen:
Bi4O6+, a Possible Reactive Center
for Alkene Oxidation"
J. Phys. Chem. A 104
(2000) 6979-82